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Minerals 2021, 11, 1330 Minerals 2021, 11, 1330 Minerals 2021, 11, 1330 same, with a small fluctuation and obvious positive correlation (Figure 14). Under certain 18 of 24 18 of 24 conditions, Mg in granite is correlated with S, while Mg in basalt is negatively correlated with Ca, K, Sr, and Li. The maximum dissolution amounts of K, Li, Mg, Ca, and S are reached after 3 h of reaction, and the maximum dissolution amount of K, Mg, S, and Br in the reaction fluid medium was distilled water or 1 mol/L NaCl solution; it reached a tghreanrietaecitsiorneafclhueid amftedri5umh owfaresadctiisotinlle(Fdigwuarete1r4o).rT1hemroels/uLltNoafCthlisorleuatciotino;nitisrqeaucithee1d7iofaf-23 maximum value of 0.152 mg/L at 250–300 °C, with a small fluctuation, and then it de- mferaexnimtfurmomvathluaetof0th.1e52brminge/Lsaamtp25le0s–3in00th°Ce,JwianitghliangsmBalslinfl,uwctuhiacthionin,daincdatethsetnhaitdthee- creased gradually with increasing temperature (Figure 16). cforermasaetdiognraodfubarlilnyeworitehtainkcerseaslionnggtetimpee. rature (Figure 16). Considering the elemental composition of the original rock, whether the reaction Considering the elemental composition of the original rock, whether the reaction fluid medium was distilled water or 1 mol/L NaCl solution, Li dissolution in basalt and fluid medium was distilled water or 1 mol/L NaCl solution, Li dissolution in basalt and granite reached a relatively high value at 250 °C, and the dissolution decreased with in- granite reached a relatively high value at 250 °C, and the dissolution decreased with in- creasing temperature. At 400 °C, the dissolution reached the lowest maximum value, creasing temperature. At 400 °C, the dissolution reached the lowest maximum value, 19.490 mg/L (Figure 16). The amount of Li in the same fluid was different at different 19.490 mg/L (Figure 16). The amount of Li in the same fluid was different at different temperatures. At the same temperature, the Li dissolution amount in the 1 mol/L NaCl temperatures. At the same temperature, the Li dissolution amount in the 1 mol/L NaCl solution was higher than that in distilled water. The dissolved Li from granite was an solution was higher than that in distilled water. The dissolved Li from granite was an order of magnitude higher than that from basalt, whether the reaction fluid medium was order of magnitude higher than that from basalt, whether the reaction fluid medium was distilled water or 1 mol/L NaCl solution; it reached the maximum value of 3.525 mg/L distilled water or 1 mol/L NaCl solution; it reached the maximum value of 3.525 mg/L at250–350 °C, with a large fluctuation, and then it decreased gradually with increasing at250–350 °C, with a large fluctuation, and then it decreased gradually with increasing temperature (Figure 16). temperature (Figure 16). The contents of Ca, Mg, and Sr in the 1 mol/L NaCl solution and distilled water de- Figure 14. Diagram of element content over time in igneous rock water–rock reaction. Figure 14. DiagrTahmeocfoenlteemnetsntocfoCntae,nMt ogv,earntidmSerininigthneo1usmrocl/kLwNaateCr–lrsoclkurteioanctiaond. distilled water de- creased with increasing temperature, and the decreasing rate of Mg was higher than that creased with increasing temperature, and the decreasing rate of Mg was higher than that 5o.f3C.3a.IannfldueSnrc(eFiogfuTrem17p)e.rHatouwrevoenrt,htheeIgcnoenotuenstRofcvkaWrioautesr–ioRnosckinR1eamcotilo/LnNaClsolution of Ca and Sr (Figure 17). However, the content of various ions in 1 mol/L NaCl solution 5.3.3. Influence of Temperature on the Igneous Rock Water–Rock Reaction was higher than that in distilled water. The content of Br in the fluid was different at was hCiognhseirdethrianngtthaet einlemdiesntitlaleldcowmapteors.itTiohne coofnttheentoorifgBinrailnrothcke,fwluhidethwearstdhieffreeraecnttioant Considering the elemental composition of the original rock, whether the reaction fluid different temperatures. At the same temperature, the content of Br ions in 1 mol/L NaCl dfliuffideremntedteiummpewraatusrdesis.tAilltetdhewsatmere oterm1pemraotlu/LreN, tahCelcosonltuentitoonf, BKr idoinssoilnut1iomnoiln/LbNasaaCltl medium was distilled water or 1 mol/L NaCl solution, K dissolution in basalt reached a solution was higher than that in distilled water (Figure 17). sreoaluchtieodn awraeslahtiigvheelyr thiagnh tvha◦altuienadtis2t5il0le°dCw, aantdert(hFeigduirseso1l7u)t.ion decreased with increasing relatively high value at 250 C, and the dissolution decreased with increasing temperature. The above analysis shows that the rates of water–rock reactions are different at dif- tempTehr◦aetuabreo.vAeta4n0a0ly°sCis, tsheodwisstohlauttitohne reaatecsheodf wthaetelor–wreosctkmreaaxcimtiounms avraeludeif,f5e4re.6n2t9amt dgi/fL- At 400 C, the dissolution reached the lowest maximum value, 54.629 mg/L (Figure 15). ferent temperatures for the same fluid. The dissolution rates of Ca, Mg, and Sr decrease f(eFrigenutrete1m5)p.eTrhaetuarmesofuonrttohfeKsainmtehfelusaidm.eThfleuidiswsoalsudtioffnereantetsatodfiCffae,reMngt,teamndpeSrratduercerse.aAset The amount of K in the same fluid was different at different temperatures. At the same with increasing temperature, while the dissolution rates of K and Li first increase and wthiethsainmceretaesminpgertaetmupre,rathtuerKe, dwihssiloelutthieondiasmsoolutnitoninra1temsool/fLKNaanCdlLsoilfuirtsiotninwcraesasheigahnedr temperature, the K dissolution amount in 1 mol/L NaCl solution was higher than that in then decrease with the increase in temperature. The change of Br is not obvious (Figure thean tdheactreinasdeiswtiiltlhedthweaitnecrr. eTahse dinissteomluptieornataumreo.uTnhteocfhLainingebaosfaBltrwisansovteorybvloiowu,sw(Fhiegtuhreer distilled water. The dissolution amount of Li in basalt was very low, whether the reaction 17). However, the content of each element in the saline fluid is much higher than that in 17). However, the content of each element in the saline fluid is much higher than that in fluid medium was distilled water or 1 mol/L NaCl solution; it reached a maximum value the distilled water, indicating that the saline fluid more easily activates ions. Basalt is the distilled water, indicating that the saline fluid more easily activates ions. Basalt is of 0.152 mg/L at 250–300 ◦C, with a small fluctuation, and then it decreased gradually with favorable for the dissolution of potassium, and granite is favorable for the dissolution of favorable for the dissolution of potassium, and granite is favorable for the dissolution of increasing temperature (Figure 16). lithium. lithium. Figure 15. Diagram of K ion content over temperature in water–rock reaction. Figure 15. Diagram of K ion content over temperature in water–rock reaction. Figure 15. Diagram of K ion content over temperature in water–rock reaction. Figure 16. Diagram of Li ion content over temperature in water–rock reaction. Figure 16. Diagram of Li ion content over temperature in water–rock reaction. Figure 16. Diagram of Li ion content over temperature in water–rock reaction. Considering the elemental composition of the original rock, whether the reaction fluid medium was distilled water or 1 mol/L NaCl solution, Li dissolution in basalt and granite reached a relatively high value at 250 ◦C, and the dissolution decreased with increasing temperature. At 400 ◦C, the dissolution reached the lowest maximum value, 19.490 mg/L (Figure 16). The amount of Li in the same fluid was different at different temperatures. AtPDF Image | Origin of Lithium Potassium Rich Brines in the Jianghan
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