Phonon-mediated quantum Hall transport in graphene

PDF Publication Title:

Phonon-mediated quantum Hall transport in graphene ( phonon-mediated-quantum-hall-transport-graphene )

Previous Page View | Next Page View | Return to Search List

Text from PDF Page: 005

Article https://doi.org/10.1038/s41467-023-35986-3 scattering mechanisms underlying the activated resistivity, in SI (Figs. S7 and S8) we discuss additional data at lower temperature (down to 50 K) and magnetic field (down to 1 T). We find that ρD drastically increases toward low T, with the activated resistivity exceeding the e-ph limit by more than one order of magnitude in a clean sample. However, as the temperature and magnetic field are increased, ρD progressively drops (i.e., the activated resistivity tends toward the e-ph limit), suggesting a temperature-driven crossover between regimes dominated by either disorder or e-ph interaction (the latter being realized only close to RT). While it is not surprising that the e-ph limit works as a lower bound to the activated resistivity of real samples, the non-universality (i.e., the sample and temperature dependence) of the disorder contribution deserves particular atten- tion in future theoretical treatments of the RT-QH in graphene. Discussion The physics of graphene is essentially determined by its deviations from flatness (that is, ripples), due to either thermal fluctuations associated to flexural phonons for freely suspended samples or to roughness of substrate like for graphene on SiO215. In both cases, rip- ples induce inhomogeneity of electron density with electron and hole puddles in the vicinity of the CNP38,39. In particular, for the case of graphene on SiO2 the amplitude of induced inhomogeneity of charge- carrier density is estimated as 3 × 1011 cm–239, in agreement with the above cited experimental values of n*. This makes the system strongly disordered, and any intrinsic scattering mechanisms become irrele- vant. Oppositely, the hBN substrate is atomically flat1 and at the same time suppresses intrinsic ripples which increases the RT carrier mobility by an order of magnitude and makes intrinsic scattering mechanisms dominant15. Indeed, experimentally measured n* for our samples is an order-of-magnitude smaller than what is supposed to be induced by ripples at RT. This results in an essentially different picture of QH physics at high enough temperatures. In conclusion, we showed experimental evidence of predominant e-ph scattering in the QH regime. This is realized by uniquely com- bining strong magnetic fields, high temperatures and hBN- encapsulation of graphene. Although the RT-QH in graphene has long been known, we showed that mitigation of disorder via van der Waals engineering provides novel insights on the transport mechan- isms in this phenomenon. Methods Graphene-hBN van der Waals assembly and device fabrication hBN/graphene/hBN samples D1-3 are assembled using the standard van der Waals dry pick-up5, starting from micromechanically exfoliated graphene flakes previously identified by optical and Raman micro- scopy. Sample D4 is obtained by CVD growth on Cu foil and direct hBN- mediated pick-up after controlled decoupling via Cu surface oxidation31. All the devices are fabricated making use of electron beam lithography, reactive ion etching and e-beam evaporation of Cr/Au 1D edge contacts5. Magnetotransport measurements We use standard lock-in acquisition at low frequency (13 Hz), with simultaneous ρxx and ρxy measurements in four-probe configuration, either under a constant current excitation (12.5 nA, sample D1-D3) or a constant voltage bias (300 μV, sample D4). The devices are mounted in a VTI system with low-pressure 4He serving as exchange gas, coupling the samples to a liquid-N2 reservoir. The cryogenic system is accom- modated in the access bore of a resistive Bitter magnet at HFML-EMFL, with a maximum field of 33 T. Reporting summary Further information on research design is available in the Nature Portfolio Reporting Summary linked to this article. Data availability The data presented in this study are available at https://doi.org/10. 5281/zenodo.7352031. References 1. Yankowitz, M., Ma, Q., Jarillo-Herrero, P. & LeRoy, B. J. van der Waals heterostructures combining graphene and hexagonal boron nitride. Nat. Rev. Phys. 1, 112–125 (2019). 2. Rhodes, D., Chae, S. H., Ribeiro-Palau, R. & Hone, J. Disorder in van der Waals heterostructures of 2D materials. Nat. Mater. 18, 541–549 (2019). 3. Bandurin, D. A. et al. Negative local resistance caused by viscous electron backflow in graphene. Science 351, 1055–1058 (2016). 4. Crossno, J. et al. Observation of the Dirac fluid and the breakdown of the Wiedemann–Franz law in graphene. Science 351, 1058–1061 (2016). 5. Wang, L. et al. One-dimensional electrical contact to a two- dimensional material. Science 342, 614–617 (2013). 6. Hwang, E. H. & Das Sarma, S. Acoustic phonon scattering limited carrier mobility in two-dimensional extrinsic graphene. Phys. Rev. B 77, 115449 (2008). 7. Sohier, T. et al. Phonon-limited resistivity of graphene by first- principles calculations: Electron-phonon interactions, strain- induced gauge field, and Boltzmann equation. Phys. Rev. B 90, 125414 (2014). 8. Park, C.-H. et al. Electron–phonon interactions and the intrinsic electrical resistivity of graphene. Nano Lett. 14, 1113–1119 (2014). 9. Morozov, S. V. et al. Giant intrinsic carrier mobilities in graphene and its bilayer. Phys. Rev. Lett. 100, 016602 (2007). 10. Chen, J.-H., Jang, C., Xiao, S., Ishigami, M. & Fuhrer, M. S. Intrinsic and extrinsic performance limits of graphene devices on SiO2. Nat. Nanotechnol. 3, 206 (2008). 11. Sonntag, J. et al. Excellent electronic transport in heterostructures of graphene and monoisotopic boron-nitride grown at atmospheric pressure. 2D Mater. 7, 031009 (2020). 12. Shi, W. et al. Reversible writing of high-mobility and high-carrier- density doping patterns in two-dimensional van der Waals hetero- structures. Nat. Electron. 3, 99–105 (2020). 13. Castro, E. V. et al. Limits on charge carrier mobility in suspended graphene due to flexural phonons. Phys. Rev. Lett. 105, 266601 (2010). 14. Polshyn, H. et al. Large linear-in-temperature resistivity in twisted bilayer graphene. Nat. Phys. 15, 1011–1016 (2019). 15. Katsnelson, M. I. The Physics of Graphene, 2nd ed. (Cambridge Uni- versity Press, 2020). 16. Klitzing, K., Dorda, G. & Pepper, M. New method for high-accuracy determination of the fine-structure constant based on quantized hall resistance. Phys. Rev. Lett. 45, 494 (1980). v. 17. Novoselov, K. S. et al. Room-temperature quantum hall effect in graphene. Science 315, 1379 (2007). 18. Jiang, Z., Zhang, Y., Tan, Y.-W., Stormer, H. L. & Kim, P. Quantum hall effect in graphene. Solid State Commun. 143, 14–19 (2007). 19. Jiang, Z., Zhang, Y., Tan, Y.-W., Stormer, H. L. & Kim, P. Quantum hall states near the charge-neutral dirac point in graphene. Phys. Rev. Lett. 99, 106802 (2007). 20. Giesbers, A. J. M. et al. Quantum-hall activation gaps in graphene. Phys. Rev. Lett. 99, 206803 (2007). 21. Ando, T., Fowler, A. B. & Stern, F. Electronic properties of two- dimensional systems. Rev. Mod. Phys. 54, 437 (1982). 22. Polyakov, D. G. & Shklovskii, B. I. Activated conductivity in the quantum hall effect. Phys. Rev. Lett. 73, 1150 (1994). 23. Polyakov, D. G. & Shklovskii, B. I. Universal prefactor of activated conductivity in the quantum hall effect. Phys. Rev. Lett. 74, 150 (1995). Nature Communications | (2023)14:318 5

PDF Image | Phonon-mediated quantum Hall transport in graphene

phonon-mediated-quantum-hall-transport-graphene-005

PDF Search Title:

Phonon-mediated quantum Hall transport in graphene

Original File Name Searched:

s41467-023-35986-3.pdf

DIY PDF Search: Google It | Yahoo | Bing

Salgenx Redox Flow Battery Technology: Power up your energy storage game with Salgenx Salt Water Battery. With its advanced technology, the flow battery provides reliable, scalable, and sustainable energy storage for utility-scale projects. Upgrade to a Salgenx flow battery today and take control of your energy future.

CONTACT TEL: 608-238-6001 Email: greg@infinityturbine.com (Standard Web Page)