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22. Lowe MA, Gao J, Abruña HD. Mechanistic insights into operational lithium–sulfur batteries by in situ X-ray diffraction and absorption spectroscopy. RSC Adv 4, 18347-18353 (2014). 23. Zhang G, et al. The Radical Pathway Based on a Lithium-Metal-Compatible High-Dielectric Electrolyte for Lithium–Sulfur Batteries. Angew Chem, Int Ed 57, 16732-16736 (2018). 24. Lodovico L, Varzi A, Passerini S. Radical Decomposition of Ether-Based Electrolytes for Li- S Batteries. J Electrochem Soc 164, A1812-A1819 (2017). 25. Yim T, et al. Effect of chemical reactivity of polysulfide toward carbonate-based electrolyte on the electrochemical performance of Li–S batteries. Electrochim Acta 107, 454-460 (2013). 26. Zou Q, Lu Y-C. Solvent-Dictated Lithium Sulfur Redox Reactions: An Operando UV–vis Spectroscopic Study. J Phys Chem Lett 7, 1518-1525 (2016). 27. Cuisinier M, Hart C, Balasubramanian M, Garsuch A, Nazar LF. Radical or Not Radical: Revisiting Lithium–Sulfur Electrochemistry in Nonaqueous Electrolytes. Adv Energy Mater 5, 1401801 (2015). 28. Pan H, et al. On the Way Toward Understanding Solution Chemistry of Lithium Polysulfides for High Energy Li–S Redox Flow Batteries. Adv Energy Mater 5, 1500113 (2015). 29. Ueno K, et al. Anionic Effects on Solvate Ionic Liquid Electrolytes in Rechargeable Lithium–Sulfur Batteries. J Phys Chem C 117, 20509-20516 (2013). 30.Fan FY, Chiang Y-M. Electrodeposition Kinetics in Li-S Batteries: Effects of Low Electrolyte/Sulfur Ratios and Deposition Surface Composition. J Electrochem Soc 164, A917-A922 (2017). 31. Elazari R, Salitra G, Garsuch A, Panchenko A, Aurbach D. Sulfur-Impregnated Activated Carbon Fiber Cloth as a Binder-Free Cathode for Rechargeable Li-S Batteries. Adv Mater 23, 5641-5644 (2011). 32. Markevich E, Salitra G, Rosenman A, Talyosef Y, Chesneau F, Aurbach D. The effect of a solid electrolyte interphase on the mechanism of operation of lithium–sulfur batteries. J Mater Chem A 3, 19873-19883 (2015). Page 22 of 24PDF Image | A lithium-sulfur battery with a solution-mediated pathway
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