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Nanomaterials 2021, 11, 810 Nanomaterials 2021, 11, x 19 of 29 Figure 13. (A) Low- and (B) high-magnification SEM images and (C) TEM image of the Ti–Nb2O5 Figure 13. (A) Low- and (B) high-magnification SEM images and (C) TEM image of the Ti–Nb2O5 NFs; (D) Operating principle of the magnesium-ion dual-ion battery and (E) its long-term cycling NFs; (D) Operating principle of the magnesium-ion dual-ion battery and (E) its long-term cycling performance at 3C with Ti–Nb2O5 NFs as anode. Adapted with permission from [177]. Copyright performance at 3C with Ti–Nb2O5 NFs as anode. Adapted with permission from [177]. Copyright American Chemical Society, 2020. American Chemical Society, 2020. 18 of 28 4.5. Other Materials 4.5. Other Materials In this section, we list other metals (and related compounds) used in the last two In this section, we list other metals (and related compounds) used in the last two years years as anodes for MIBs. It is important to underline that also computational chemistry as anodes for MIBs. It is important to underline that also computational chemistry aims aims to predict new promising compounds as anodes for MIBs; some of these examples to predict new promising compounds as anodes for MIBs; some of these examples are are discussed below. discussed below. Zhang et al. prepared VO2 NWs by a conventional hydrothermal process [183]; their Zhang et al. prepared VO2 NWs by a conventional hydrothermal process [183]; their width was uniformly distributed around 100–300 nm and the length was equal to ≈ 10 μm width was uniformly distributed around 100–300 nm and the length was equal to ≈ 10 μm (F(Figiguurere114B4B).)T. Thhisiseleelcetcrtordode ewwasasfifrisrtstetsetsetdedininaaMggSSOO411.0.0Maaqquueeoouusseelelecctrtorolylytete, ,sshhoowwiningg 4 ininitiitaiallchchaargrgeeddcacappaacictiiteiesseqequuaalltoto26236,32,0270.7.,71,4164.64.4anadnd10130m3 mAAhhgg aatt11000,,22000,,55000anandd −1−1 110000m mA g ,,reressppeecctitviveelyly..CConovnevresresleyl,yp, epreforfromrmanacnecseisniMn gMCgl2C-lan-danMdgM(NgO(N3)2O-ba)s-ebdaseeledc- −11 etlreocltyrotelystwesewreeraethraetrhperoopro,othr,uthsushsoswhoinwgi—nga—gaignaintihnethMeIMBsIBfiselfide—ldt—hethrelreevlaenvtanrotlreooleftohfe 232 thmeamgnaegsniuesmiusmalstaflotrfoerleecltercotlryotleytfeorfmorumlautliaotnio.nA.sAcsoncocnercnesrnpsrpolronlognegdecdhcahragreg/de/isdcihsacrhgaergeex- −1 epxepreirmimenetnstasta5t005 0m0Am gA ,gthe,VtOhe2 NVWOs rNevWeaslerdevaecaylecdlinagcsytacbliinligtysotafb5i4li.3ty%oafft5e4r.130%0 cayftcelers −1 2 1(0F0igcyucrles14(FAig);usruec1h4aAn);imsupchoratnanimt fpadorintagnwt fasdainttgriwbuatseadtttroibtuhteepdatrotitahlelypiarrteivalelrysirbrlevrerascibtiloen reoafcmtioagnnoefsmiuamgnioesnisu(mnoiotnbsei(ngotfubleliyngexfturlalcytedxtfrraocmtedthfreohmostthmehaotesrtimalaltaetrticael)latntidcet)haenpdatrhtieal pdairstsiaolludtiisosnoluotfioVnOo2fiVnOtheineltehcetreolleycteroulyptoenutpiomnet.iEmvee.nEvimenprimovpermoveenmtsewntesrweerreequreiqreudir,etdh,e 2 the authors were able to follow the mechanism of the reaction by different characterization authors were able to follow the mechanism of the reaction by different characterization techniques.Indetail,VO transformedintoastableMgVO structureafterthefirstcharge, techniques. In detail, VO22 transformed into a stable MgVOxx structure after the first charge, then the insertion/extraction of magnesium ions was accompanied by the valence changes then the insertion/extraction of magnesium ions was accompanied by the valence changes 5+ 4+ 4+ 3+ of V 5+ (reduced to V 4+ ) and V4+ (reduced to V3+ ). ofV (reducedtoV )andV (reducedtoV ).PDF Image | Overview on Anodes for Magnesium Batteries
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