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Batteries 2022, 8, 59 14 of 17 References (7) which is instrumental in increasing the electronic conductivity and suppression of Zn dendrites. However, the fundamental mechanism of interfacial reaction between the polymer electrolytes and electrodes is still insufficient. Furthermore, the SEI is usually affected and destroyed by the surface topography changes of the Zn anode due to dendrite growth. Further research efforts should be dedicated to the stabilization of the SEI. Multifunctional polymer electrolytes can effectively broaden the application range of flexible Zn-based batteries to satisfy diverse application requirements. Some in- triguing functionalities, such as extreme temperature tolerance, thermoresponsive properties, and self-healing ability have been summarized in the preceding sections. Many other potential functionalities, including photodetection, electrochromism, and shape memory are also worthy of exploration for the development of advanced flexible batteries. In addition, the integration of flexible Zn-based batteries with other wearable device systems, such as sensors, self-powering generators, and energy conversion devices has been identified as a promising direction for next-generation wearable electronics. Author Contributions: F.M., B.G. and W.L. contributed equally to the literature search and drafted the majority of this paper; G.L. contributed to the manuscript design and refinement; J.W. and L.C. revised the paper; S.Y. conducted the literature screening. All authors have read and agreed to the published version of the manuscript. Funding: The authors gratefully acknowledge the financial support of Shenzhen Municipality un- der Project of Scientific Research Foundation for Returned Scholars (Grant No. DD11409018). This research was also sponsored by the Shenzhen Science and Technology Program (Grant No. KQTD20200820113045083). Institutional Review Board Statement: Not applicable. Informed Consent Statement: Not applicable. Data Availability Statement: Not applicable. Conflicts of Interest: The authors declare no conflict of interest. 1. Li, Y.; Fu, J.; Zhong, C.; Wu, T.; Chen, Z.; Hu, W.; Amine, K.; Lu, J. Recent Advances in Flexible Zinc-Based Rechargeable Batteries. Adv. Energy Mater. 2019, 9, 1802605. [CrossRef] 2. Yu, P.; Zeng, Y.; Zhang, H.; Yu, M.; Tong, Y.; Lu, X. Flexible Zn-Ion Batteries: Recent Progresses and Challenges. Small 2019, 15, 1804760. [CrossRef] [PubMed] 3. Zhao, Y.; Guo, J. Development of Flexible Li-Ion Batteries for Flexible Electronics. InfoMat 2020, 2, 866–878. [CrossRef] 4. Qian, G.; Liao, X.; Zhu, Y.; Pan, F.; Chen, X.; Yang, Y. Designing Flexible Lithium-Ion Batteries by Structural Engineering. ACS Energy Lett. 2019, 4, 690–701. [CrossRef] 5. Kim, T.; Song, W.; Son, D.-Y.; Ono, L.K.; Qi, Y. Lithium-Ion Batteries: Outlook on Present, Future, and Hybridized Technologies. J. Mater. Chem. A 2019, 7, 2942–2964. [CrossRef] 6. Xiong, R.; Pan, Y.; Shen, W.; Li, H.; Sun, F. Lithium-Ion Battery Aging Mechanisms and Diagnosis Method for Automotive Applications: Recent Advances and Perspectives. Renew. Sustain. Energy Rev. 2020, 131, 110048. [CrossRef] 7. Han, X.; Lu, L.; Zheng, Y.; Feng, X.; Li, Z.; Li, J.; Ouyang, M. A Review on the Key Issues of the Lithium Ion Battery Degradation among the Whole Life Cycle. ETransportation 2019, 1, 100005. [CrossRef] 8. Tang, B.; Shan, L.; Liang, S.; Zhou, J. Issues and Opportunities Facing Aqueous Zinc-Ion Batteries. Energy Environ. Sci. 2019, 12, 3288–3304. [CrossRef] 9. Fang, G.; Zhou, J.; Pan, A.; Liang, S. Recent Advances in Aqueous Zinc-Ion Batteries. ACS Energy Lett. 2018, 3, 2480–2501. [CrossRef] 10. Blanc, L.E.; Kundu, D.; Nazar, L.F. Scientific Challenges for the Implementation of Zn-Ion Batteries. Joule 2020, 4, 771–799. [CrossRef] 11. Zhang, N.; Chen, X.; Yu, M.; Niu, Z.; Cheng, F.; Chen, J. Materials Chemistry for Rechargeable Zinc-Ion Batteries. Chem. Soc. Rev. 2020, 49, 4203–4219. [CrossRef] [PubMed] 12. Shin, J.; Lee, J.; Park, Y.; Choi, J.W. Aqueous Zinc Ion Batteries: Focus on Zinc Metal Anodes. Chem. Sci. 2020, 11, 2028–2044. [CrossRef] [PubMed]PDF Image | Flexible Zn-Based Batteries with Polymer Electrolyte
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