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11 4.A methodassetforthinclaim1whereintheformate dehydrogenase, formaldehyde dehydrogenase and alcohol dehydrogenase enzymes are ?xed in a microporous matrix. 5. A method as set forth in claim 4 Wherein the microporous matrix is a sol-gel matrix. 6.A methodassetforthinclaim1Whereintheterminal electron donor is reduced nicotinamide adenine dinucle otide. 7.A methodassetforthinclaim5Whereintheterminal electrondonorisreducednicotinamideadeninedinucle 10 otide. 12 nicotinamide adenine dinucleotide by contacting the nicoti namide adenine dinucleotide With hydrogen. 16. A method as set forth in claim 9 Wherein the sol-gel matrixiselectroactiveandthesol-gelmatrixregeneratesthe reduced nicotinamide adenine dinucleotide from the nicoti namide adenine dinucleotide. 17.A methodforreductionofformaldehydetomethanol by alcohol dehydrogenase catalysis, comprising exposing alcohol dehydrogenase enZymes retained in a microporous matrix to the formaldehyde. 18. A method as set forth in claim 17 Wherein the formaldehyde is produced by reduction of formate to the formaldehyde by formaldehyde dehydrogenase catalysis, US 6,440,711B1 8.A methodassetforthinclaim6Whereinthereduced nicotinamide adenine dinucleotide is oxidiZed to nicotina mide adenine dinucleotide upon donation of a terminal electron and is regenerated back to reduced nicotinamide 15 comprisingexposingformaldehydedehydrogenaseenZymes adenine dinucleotide to serve again as a terminal electron donor. 9.A methodassetforthinclaim7Whereinthereduced nicotinamide adenine dinucleotide is oxidiZed to nicotina mide adenine dinucleotide upon donation of a terminal electron and is regenerated back to reduced nicotinamide adenine dinucleotide to serve again as a terminal electron donor. 10.Amethod assetforthinclaim8Whereinthereduction ofthecarbondioxidetomethanoltakesplaceinWaterand 25 the reduced nicotinamide adenine dinucleotide is regener ated by a photosystem preparation exposed to light. 11.Amethod assetforthinclaim9Whereinthereduction of the carbon dioxide to methanol takes place in Water and the reduced nicotinamide adenine dinucleotide is regener ated by a photosystem preparation exposed to light. 12. A method as set forth in claim 10 Wherein the photosystem preparation isaphotosystem Ipreparation. retained in a microporous matrix to the formate. 19.Amethod assetforthinclaim18Whereintheformate isproducedbyreductionofcarbondioxidetotheformateby formatedehydrogenasecatalysis,comprisingexposingfor mate dehydrogenase enZymes retained in a microporous matrix to the carbon dioxide. 20. A method as set forth in claim 17 Wherein reduced nicotinamide adenine dinucleotide acts as a terminal elec tron donor in the reduction. 21. A method as set forth in claim 18 Wherein reduced nicotinamide adenine dinucleotide acts as a terminal elec tron donor in each of the reductions. 22. A method as set forth in claim 19 Wherein reduced nicotinamide adenine dinucleotide acts as a terminal elec tron donor in each of the reductions. 23.A methodassetforthinclaim22Whereinthereduced nicotinamide adenine dinucleotide is oxidiZed to nicotina mide adenine dinucleotide upon donation of terminal elec tron to the reductions and is regenerated back to reduced 13. A method as set forth in claim 11 Wherein the photosystempreparationisaphotosystemIpreparation. 35 nicotinamide adenine dinucleotide to serve again as a ter 14. A method as set forth in claim 8 Wherein the nicoti namide adenine dinucleotide is regenerated back to reduced nicotinamide adenine dinucleotide by contacting the nicoti namide adenine dinucleotide With hydrogen. 15. A method as set forth in claim 9 Wherein the nicoti namide adenine dinucleotide is regenerated back to reduced minal electron donor for further reduction reactions. 24.A methodassetforthinclaim2Whereintheformate dehydrogenase, formaldehyde dehydrogenase and alcohol dehydrogenase enZymes are ?xed in a microporous matrix.PDF Image | DEHYDROGENASE ENZYMATIC SYNTHESIS OF METHANOL
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