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UnitedStatesPatent [19] Steinbergeta]. [54] METHOD FOR CONVERTING NATURAL GAS AND CARBON DIOXIDE TO METHANOL AND REDUCING CO, EMISSIONS [76] Inventors: MeyerSteinberg.15Alder?eldLa.. Melville.NY. 11747;YuanjiDong. 101-1ASpringsetDr..Cary.NC. 27513 [21] Appl.No.:583,315 [22] Filed: Jan.5,1996 Related US. Application Data [63] Continuation-impart of Ser. No. 405,032, Mar. 16, 1995, abandoned. [51] Int(:1.6..C07C27/06 [52] US.Cl...518/703;518/702;518/704; 518/705;423/453;423/458 [58] FieldofSearch ..518/702.703. 518/704. 705; 423/453. 458 [56] References Cited U.S. PATENT DOCUMENTS 1,803,221 4/1931 Tyrereta1.. 5,529,599 6/1996 Calderon ..............................75/1063 US005767165A [1] PatentNumber: 5,767,165 [45] DateofPatent: Jun.16,1998 OTHER PUBLICATIONS Kirk-Othmer Encyclopedia of Chemical Technology.vol. 12.p.965. 1978. Kirk-Othmer Encyclopedia of Chemical Technologyvol. 15.1.400. 1978. Primary Examiner-Gary Geist AssistantExaminer--S. Padrnanabhan Attorney,Agent,orFirm-Kelly& Hulrne.RC. [57] ABSTRACT A processfortheproductionofmethanolfromnaturalgas containingmethanecomprisingthethermaldecomposition of methane and the subsequent reaction of the resulting hydrogen gas with carbon dioxide in a catalyst containing methanol synthesis reactor to produce methanol. Alternative methods include the gasi?cation with carbon dioxide of at least a portion of the carbon produced by the decomposing step. to produce carbon monoxide. which is then reacted withhydrogengastoproducemethanol;orthereformingof a portion of the natural gas feedstock used in the decom posing step With carbon dioxide to produce carbon monox ide and hydrogen gas. which carbon monoxide and hydro gen are then combined with additional hydrogen from the natural gas decomposing step in a methanol synthesis reac tor to produce methanol. The methods taught reduce the overall amount of carbon dioxide resulting from the metha nolproductionprocess. 2Claims,2DrawingSheetsPDF Image | CONVERTING NATURAL GAS AND CARBON DIOXIDE TO METHANOL
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