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Figure 4-37. Schematic summary of the proposed mechanism for Li2S activation during initial charge. A complete metallic lithium-free, Si/Li2S cell was also presented and promising results were obtained. The cycling properties were very close to the one obtained with Li, thus further improvement of Si/Li2S cell may bring additional benefits. Utilization of graphite with sulfur and/or Li2S-based electrodes would be difficult to achieve, mostly due to the incompatibility of graphite with ether-based electrolytes. We have demonstrated that, indeed, even if using little amount of VC additive in ether-based electrolyte, we could not achieve stable cyclability of the graphite electrode. On the contrary, silicon electrode seems to be a promising choice for the Li/S system. 156 Chapter 4: Li2S electrodePDF Image | Accumulateur Lithium Soufre
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